TY - JOUR AU - Koehler, Jens AU - Wollenhaupt, Matthias AU - Bayer, Tim AU - Sarpe, Cristian AU - Baumert, Thomas T1 - Zeptosecond precision pulse shaping JO - OPTICS EXPRESS PY - 2011/jun 6 VL - 19 IS - 12 SP - 11638 EP - 11653 UR - DO - KW - imported L1 - SN - N1 - N1 - AB - We investigate the temporal precision in the generation of ultrashort

laser pulse pairs by pulse shaping techniques. To this end, we combine a

femtosecond polarization pulse shaper with a polarizer and employ two

linear spectral phase masks to mimic an ultrastable common-path

interferometer. In an all-optical experiment we study the interference

signal resulting from two temporally delayed pulses. Our results show a

2 sigma-precision of 300 zs = 300 x 10(-21) s in pulse-to-pulse delay.

The standard deviation of the mean is 11 zs. The obtained precision

corresponds to a variation of the arm's length in conventional delay

stage based interferometers of 0.45 angstrom. We apply these precisely

generated pulse pairs to a strong-field quantum control experiment.

Coherent control of ultrafast electron dynamics via photon locking by

temporal phase discontinuities on a few attosecond timescale is

demonstrated. (C) 2011 Optical Society of America ER -